Direct probing of temperature-independent bulk half-metallicity in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>Co</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:mi>MnSi</mml:mi></mml:mrow></mml:math> by spin-resolved hard x-ray photoemission
نویسندگان
چکیده
We have performed the bulk-sensitive spin-resolved hard x-ray photoelectron spectroscopy (HAXPES) to directly clarify spin-dependent valence band electronic states and spin polarization of $L{2}_{1}$-ordered ${\mathrm{Co}}_{2}\mathrm{MnSi}$ as a predicted half-metal. The HAXPES spectra clearly exhibited difference in majority minority bulk region 30-nm-thick ${\mathrm{Co}}_{2}\mathrm{MnSi}(001)$ thin film buried under MgO(2 nm) layer at both temperatures 21 300 K. As expected from half-metallicity ${\mathrm{Co}}_{2}\mathrm{MnSi}$, we found that (minority) spectrum shows metallic Fermi edge (a gap), leading high \ensuremath{\sim}90% around level temperature experiments revealed is independent on up also slight changes spectral shapes shift maximum with temperature. By comparing experimental results first-principles calculations finite obtained by disordered local moment method, it suggested mainly caused temperature-dependent Co $3d$ states. It conduction minimum located sufficiently above
منابع مشابه
Probing bulk electronic structure with hard X-ray angle-resolved photoemission.
Traditional ultraviolet/soft X-ray angle-resolved photoemission spectroscopy (ARPES) may in some cases be too strongly influenced by surface effects to be a useful probe of bulk electronic structure. Going to hard X-ray photon energies and thus larger electron inelastic mean-free paths should provide a more accurate picture of bulk electronic structure. We present experimental data for hard X-r...
متن کاملDevelopment of the hard-X-ray angle resolved X-ray photoemission spectrometer for laboratory use.
This article reports development of a practical laboratory hard X-ray photoelectron spectroscopy (HXPS) system by combining a focused monochromatic Cr K(alpha) X-ray source, a wide angle acceptance objective lens and a high kinetic energy electron analyzer. The Cr K(alpha) source consists of a Cr target, a 15 kV focused electron gun, and a compact bent crystal monochromator. The X-ray spot size...
متن کاملExploring the XPS limit in soft and hard x-ray angle-resolved photoemission using a temperature-dependent one-step theory
J. Braun,1 J. Minár,1 S. Mankovsky,1 V. N. Strocov,2 N. B. Brookes,3 L. Plucinski,4,5 C. M. Schneider,4,5 C. S. Fadley,6,7 and H. Ebert1 1Department Chemie, Ludwig-Maximilians-Universität München, 81377 München, Germany 2Swiss Light Source, Paul Scherrer Institut, CH 5232 Villingen, PSI, Switzerland 3European Synchrotron Radiation Facility (ESRF), Bote Postale 220, 38043 Grenoble, France 4Peter...
متن کاملBulk electronic structure of the dilute magnetic semiconductor Ga(1-x)Mn(x)As through hard X-ray angle-resolved photoemission.
A detailed understanding of the origin of the magnetism in dilute magnetic semiconductors is crucial to their development for applications. Using hard X-ray angle-resolved photoemission (HARPES) at 3.2 keV, we investigate the bulk electronic structure of the prototypical dilute magnetic semiconductor Ga(0.97)Mn(0.03)As, and the reference undoped GaAs. The data are compared to theory based on th...
متن کاملBulk electronic structure of superconducting LaRu2P2 single crystals measured by soft-X-ray angle-resolved photoemission spectroscopy.
We present a soft x-ray angle-resolved photoemission spectroscopy (SX-ARPES) study of the stoichiometric pnictide superconductor LaRu(2)P(2). The observed electronic structure is in good agreement with density functional theory (DFT) calculations. However, it is significantly different from its counterpart in high-temperature superconducting Fe pnictides. In particular, the bandwidth renormaliz...
متن کاملذخیره در منابع من
با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید
ژورنال
عنوان ژورنال: Physical review
سال: 2022
ISSN: ['0556-2813', '1538-4497', '1089-490X']
DOI: https://doi.org/10.1103/physrevb.106.075101